.Net Test Automation
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If razzie's assumption is true and you want to test your gui, if you are developing a Windows Form application, use TestComplete , its ideal tools for this use, and generally test automation.
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I'm not really sure what you want to achieve. If you want to "unit test" your GUI, for example, a user clicks on a link and he has to go to page X, then I think NUnitASP is close to what you want. You can basically say that you are navigating to page X, and then you can test various things like a textbox that should be present, what should happen when a user tries to save a form on that page, etc. See what you need.
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